生态与环境科学

不同源区大气降尘的磁学性质及其环境意义

  • 李 勇 ,
  • 邹长明 ,
  • 姚 洁
展开
  • 1. 安徽科技学院 电气与电子工程学院, 安徽 凤阳233100; 2. 安徽科技学院 资源与环境学院, 安徽 凤阳 233100
李 勇, 男, 硕士, 副教授, 研究方向为磁学和环境磁学. E-mail: liyong197510@163.com.

收稿日期: 2015-10-14

  网络出版日期: 2016-09-29

Magnetic properties of atmospheric dustfall from different source region and its environmental significance

  • LI Yong ,
  • ZOU Chang-ming ,
  • YAO Jie
Expand
  • 1. College of Electrical and Electronic Engineering, Anhui Science and Technology University, Fengyang Anhui 233100, China;
    2. College of Resource and Environment, Anhui Science and Technology University, Fengyang Anhui 233100, China

Received date: 2015-10-14

  Online published: 2016-09-29

摘要

为了研究大气降尘磁学性质对污染物来源的指示作用, 对水泥厂、石英砂厂和县城等不同源区大气降尘的磁学参数、矿物成分、微观形貌和粒度特征进行了测量,
结果表明降尘都以地方性物质为主, 石英砂厂降尘大部分是粒状单矿物, 粒度较粗, 棱角分明, 主要成分是石英; 水泥厂降尘呈片状和不规则粒状集合体, 主要矿物成分是硅酸盐和碳酸盐; 县城降尘呈粒状和絮状, 成分比较复杂, 主要元素有: Si、Al、Na、Ca、Fe~等. 降尘中磁性矿物含量随着季节变化, 冬季高于其他季节; 不同源区降尘中磁性矿物含量存在差异, 县城降尘最高, 其磁学参数对污染物来源具有良好的指示作用. 水泥厂和石英砂厂大气污染严重, 每月降尘量的平均值远高于县城,
但这2类工业降尘中磁性矿物含量比县城低, 且磁学特征相似, 需结合其矿物成分、微观形貌和粒度特征进行区分, 建立降尘与污染源之间的联系.

本文引用格式

李 勇 , 邹长明 , 姚 洁 . 不同源区大气降尘的磁学性质及其环境意义[J]. 华东师范大学学报(自然科学版), 2016 , 2016(4) : 158 -168 . DOI: 10.3969/j.issn.1000-5641.2016.04.018

Abstract

In order to study the indication effect of magnetic properties of atmospheric dustfall on the pollution source, magnetic parameters, mineral composition, morphology and particle size were measured on atmospheric dustfall from different source region of cement factory, quartz sand factory and county seat. Results showed that dustfall mainly came from the local matter, the dustfall of quartz sand factory was monomineral with morphology of granular structure, its main component was quartz with coarse grain size and angular shape. The dustfall of cement factory was sheet and irregularly granular aggregation, its principal constituents were silicates and carbonates. The dustfall of county seat was granular and flocculent, the component was complex, whose main elements were Si!Al!Na!Ca!Fe and so on. The magnetic mineral content of dustfall changed with seasons, it was higher in winter. The magnetic mineral content of dustfall from different source region was not the same, the dustfall of county seat was the highest, its magnetic parameters can be a good indicator of pollution sources. The atmosphere pollution of quartz sand factory and cement factory was serious, their average values of monthly dustfall were far higher than county seat, but the magnetic mineral content of these two kinds of industrial dustfall was lower than county seat, and their magnetic characteristics was similar. We must combine with their mineral composition, morphology and particle size to distinguish, then set up connection. 

参考文献

[1] HARRISON R M, SMITH D J T, PIO C A, et al. Comparative receptor modelling study of airborne particulate pollutants in Birmingham(United Kingdom), Coimbra(Portugal) and Lahore(Pakistan)[J]. Atmospheric Environment, 1997, 31(20): 3309-3321.
[2] 田裘学, 周伶芝. 兰州市大气污染对居民健康影响的研究 [J].中国环境科学, 1994, 14(3): 200-205.
[3] STONE E, SCHAUER J, QURAISHI T A, et al. Chemical characterization and source apportionment of fine and coarse particulate matter in Lahore, Pakista [J]. Atmospheric Environment, 2010, 44(8): 1062-1070.
[4] 尹刚, 胡守云, 闫海涛. 不同环境污染载体的磁学研究及其应用特点 [J].地球物理学进展, 2012, 27(5): 1947-1956.
[5] GAUTAM P, BLAHA U, APPEL E. Magnetic susceptibility of dust-loaded leaves as a proxy of traffic-related heavy metal pollution in Kathmandu City, Nepal [J]. Atmospheric Environment, 2005, 39(12): 2201-2211.
[6] MAHER B A, MOORE C, MATZKA J. Spatial variation in vehicle-derived metal pollution identified by magnetic and elemental analysis of roadside tree leaves [J]. Atmospheric Environment, 2008, 42(2): 364-373.
[7] MUXWORTHY A R, MATZKA J, PETERSEN N. Comparison of magnetic parameters of urban atmospheric particulate matter with pollution and meteorological data [J] Atmospheric Environment, 2001, 35(26): 4379-4386.
[8] MUXWORTHY A R, MATZKA J, DAVILA A F, et al. Magnetic signature of daily sampled urban atmospheric particles [J] Atmospheric Environment, 2003, 37(29): 4163-4169.
[9] 夏敦胜, 余晔, 马剑英, 等. 大气降尘磁学特征对城市污染源的指示 [J].干旱区资源与环境, 2007, 21(12): 110-115.
[10] 田世丽, 夏敦胜, 余晔, 等.西北地区河谷城市大气降尘环境磁学特征及其环境意义 [J]. 环境科学,2011, 32(9): 2761-2768.
[11] SHU J, DEARING J A, MORSE A P, et al. Determining the sources of atmospheric particles in Shanghai, China, from magnetic and geochemical properties [J]. Atmospheric Environment, 2001, 35: 2615-2625.
[12] 李鹏, 强小科, 徐新文, 等.西安市道路灰尘磁学特征及其对环境的响应 [J]. 地球物理学报, 2010,53(1): 156-163.
[13] 乔庆庆, 黄宝春, 张春霞.华北地区大气降尘和地表土壤磁学特征及污染来源 [J]. 科学通报, 2014,59(18): 1748-1760.
[14] 朱艳明, 郭小蕾, 周力平. 北京地区表土磁性特征及其环境意义 [J].科学通报, 2010, 55(17): 1717-1725.
[15] 夏敦胜, 杨丽萍, 马剑英, 等.中国北方城市大气降尘磁学特征及其环境意义 [J]. 中国科学: D辑, 2007,37(8): 1073-1080.
[16] 王丽, 夏敦胜, 余晔, 等.北疆地区城市大气降尘磁学特征及其环境意义 [J]. 中国沙漠, 2010, 30(3): 699-705.
[17] SHU J, DEARING A, MORSE A P, et al. Determining the sources of atmospheric particles in Shanghai, China, from magnetic and geochemical properties [J]. Atmospheric Environment, 2001, 35(15): 2615-2625.
[18] 乔庆庆, 张春霞, 李静, 等. 北京市朝阳区大气降尘磁学特征及对空气污染物浓度的指示 [J].地球物理学报, 2011, 54(1): 151-162.
[19] 王赞红. 现代尘暴降尘与非尘暴降尘的粒度特征 [J]. 地理学报, 2003,58(4): 606-610.
[20] 李晋昌, 董治宝. 大气降尘研究进展及展望 [J]. 干旱区资源与环境, 2010,24(2): 102-109.
[21] EVANS M E, HELLER F. Environmental Magnetism [M]. London: Academic Press, 2003.
[22] THOMPSON R, OLDFIELD F. Environmental Magnetism [M]. London: Allen and Unwin, 1986.
[23] YAMAZAKI T. Gautionary note on magnetic grain-size estimation using the ratio of ARM to magnetic susceptibility [J]. Geophysical Research Letters, 1997, 24(7): 751-754.
[24] HEIDER F, ZITZELSOBERGER A, FABIAN K. Magnetic susceptibility and remanent coercive force in grown magnetite crystals from 0.1$\mu $m to 6mm [J]. Physics of the Earth and Planetary Interiors, 1996, 93(3/4): 239-256.
[25] OLDFIELD F. Toward the discrimination of fine-granded ferrimagnets by magnetic measurements in lake and near shore marine sediments [J]. Journal of Geophysical Research, 1994, 99(b5): 9045-9050.
[26] DUNLOP D J, OZDEMIR O. Rock Magnetism: Fundmentals and Frontiers [M]. Cambridge: Cambridge University Press, 1997.
[27] LI H Y, ZHANG S H. Detection of mineralogical changes in pyrite using measurements of temperature-dependence susceptIhi1ities [J]. Chinese Journal of Geophysics. 2005, 48(6): 1454-146l.
[28] 王喜生, LOVLIE R, 苏朴. 许家窑泥河湾沉积物的岩石磁学性质 [J]. 中国科学(D辑), 2002,32(4): 271-278.
[29] DEARING J A, BIRD P M, DANN R J L, et al. Secondary ferrimagnetic minerals in Welsh soils: A comparison of mineral magnetic detection methods and implications for mineral formation [J]. Geophysical Journal International, 1997, 130(3): 727-736.
[30] WANG X M, DONG Z B, YAN P, et al. Surface sample collection and dust source analysis in north western China [J]. Catena, 2005, 59(1): 35-53.

文章导航

/